Open quantum systems with time-delayed interactions

Abstract

The subject of this thesis is the modelling of non-Markovian open quantum systems, in particular those that display memory effects due to time-delayed interactions. I study these systems in the context of a model of an open quantum system that interacts with a bosonic environment by way of particle exchanges. While the model is flexible enough to describe quite general memory effects, this work focuses to a large extent on a single prototypical system. This system emits into a coherent feedback loop with a time delay, and it captures the essential phenomena we aim to model. Within the context of this general model, I develop a general approach to spontaneous emission from singly-excited systems and show how to calculate the corresponding emission spectra. I also evaluate two commonly-used perturbative techniques in the context of spontaneous emission from singly-excited systems, coming to the conclusion that perturbation theory is of limited use in modelling open quantum systems with delayed feedback. I then turn attention to exact equations of motion for more general non-Markovian open quantum systems. I derive Heisenberg–Langevin equations that describe a large class of such systems, and solve these equations analytically for a series of simple bosonic systems. I also use the theory of cascaded open quantum systems to simulate systems with delayed coherent feedback in the limit of long time delay, and compare the results of these simulations with the analytic solutions obtained in the Heisenberg picture. Finally, I show that once we have a solution to a given Heisenberg–Langevin equation we can derive an alternative, time-local equation of motion that describes equivalent dynamics, and that these time-local Heisenberg–Langevin equations can in turn be used to derive corresponding time-local master equations. These master equations provide an exact description of the non-Markovian dynamics, but this treatment is limited to linear, bosonic systems—those systems for which the Heisenberg–Langevin equations can be solved in closed form. I discuss the prospect of generalising these master equations to take into account nonlinear and fermionic systems.